短短数日内，三起“微笑杀人案”震动全城。 林峰调查过程中，青年警探、警局“活宝”王不二（文章饰）语出惊人：这是一起连环谋杀案！遂与搭档黄飞红（李连杰饰)开始了一段惊悚刺激，同时又状况不断的“缉凶”之旅。黄飞红在旁边看似总是乌龙，但其实是真正的功夫高手，每到关键时刻，他总能帮助王不二化险为夷。案件侦办过程中，王不二先是将怀疑对像锁定为女明星刘金水(刘诗诗饰），随着案情的深入，刘金水的嫌疑被逐渐撇清，她的姐姐戴依依(柳岩饰）等人又成了王不二的怀疑对象。最后，王不二决定假扮刘金水的男友来引诱凶手现身。与此同时，危险也慢慢向王不二靠近，真相即将大白于天下，王不二与凶手的终极对决，也就此展开。最终，王不二看出破绽，擒获真凶，不仅还了刘金水清白，更因此收获了爱情。 刘诗诗人物简介黄飞红（李连杰饰）是一名将要退休的警员，曾经勇猛的他为了能顺利退休，想尽办法远离是非和麻烦。偏偏事与愿违，上司Angela（陈妍希 饰）将冒失冲动的王不二（文章 饰）分配给黄飞红做搭档。第一次搭档，在非法交易现场埋伏，阴差阳错放过了嫌疑人，和突然出现的逃犯陈虎（邹兆龙 饰）大打出手，破坏了原本行动计划，被上级狠狠训斥一番。接著，三人接手了棘手的“微笑离奇杀人事件”，所有死者脸上都带有诡异的神秘微笑。查案过程中黄飞红和王不二遭遇各种险情：潜入死者家搜集证据时和保险调查员（吴京 饰）大打出手；怀疑女演员刘金水（刘诗诗 饰）是情杀凶手，在电影拍摄现场抓获正在拍摄动作戏扮演杀手的刘金水，又怀疑性感的保险销售戴依依（柳岩 饰）为了巨额保险谋杀受害者。而刘金水和戴依依最终都有不在场证据，凶手却另有其人......
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